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题名/责任者:

Stable Supported Gold Nanoparticle Catalyst for Environmentally Responsible Propylene Epoxidation / by Nidhi Kapil.

版本说明:

1st ed. 2022.

出版发行项:

Cham : Springer, 2022.

ISBN:

9783031150661

ISBN:

9783031150654 (print)

ISBN:

9783031150678 (print)

ISBN:

9783031150685 (print)

载体形态项:

xxii, 197 pages : illustrations ; 24 cm

丛编说明:

Springer Theses, Recognizing Outstanding Ph.D. Research, 2190-5061

丛编统一题名:

Springer Theses, Recognizing Outstanding Ph.D. Research,

个人责任者:

Kapil, Nidhi.

附加团体名称:

SpringerLink (Online service)

论题主题:

Chemical engineering.

论题主题:

Nanotechnology.

论题主题:

Catalysis.

论题主题:

Sustainability.

中图法分类号:

TQ02

内容附注:

Introduction -- Propylene Oxide and Its Production -- Propylene Epoxidation Reactor Design -- Synthesis of Gold Cluster-Based Catalyst and Effect of Pre-Treatments on Its Catalytic Performance -- Precisely Engineered Supported Gold Clusters as a Stable Catalyst for Propylene Epoxidation -- Tailoring Gold Nanoparticles with Tunable Core Size and Their Catalytic Applications -- Propylene Epoxidation on Au/Ti-containing Supports: The Effect of the Support -- Controlled Engineering of Supported Metal Nanoparticles Using Electrospraying: Robust Removal of Stabilising Ligands -- Conclusions and Future Work -- Appendix.

摘要附注:

This book describes a detailed multi-scale approach integrating nano- (active site), meso- (porous catalyst architecture) and macroscale (reactor) efforts, to address the challenges of producing a better epoxidation catalyst. It contains an in-depth study of the design and synthesis of gold nanoparticles and their application as a catalyst for direct gas phase propylene epoxidation. "Direct" means using only hydrogen and oxygen in one step, which is key for sustainable manufacturing, as opposed to commercialised, more complex production routes requiring multiple steps, or integration with another chemical plant. The insights gained can be used for rational design for stable and selective catalysts for other reactions. It also details the step-by-step process to build an epoxidation reactor system with a focus on safety aspects, which can be used as a guidebook for undergraduate and graduate students in chemical engineering. Beyond heterogeneous catalysis, the new, easily accomplished methodology for synthesising atomically precise nanoparticles is shown to be relevant to electrocatalysis and to healthcare applications, such as anti-microbial surfaces. This book will be of interest to researchers, engineers and experts in the related areas of chemical engineering, chemistry, material science and electrochemistry.

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